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Homogeneous isolation of nanocelluloses by controlling the shearing force and pressure in microenvironment.

マイクロ環境におけるせん断力と圧力の制御によるナノセルロースの均一単離

other not specified not assessed

Abstract

Nanocelluloses were successfully isolated from sugarcane bagasse cellulose using dynamic high pressure microfluidization (DHPM), which achieved homogeneous dispersion by regulating shear forces and pressure within a microenvironment. Compared with conventional high pressure homogenization, DHPM required fewer processing cycles at elevated pressure. X-ray diffraction and X-ray photoelectron spectroscopy confirmed that entangled cellulose network structures were effectively dispersed, with intermolecular hydrogen bonds disrupted. Gel permeation chromatography, solid-state 13C NMR, and FT-IR analyses indicated that intramolecular hydrogen bonds remained intact. The resulting nanocelluloses exhibited reduced particle size, favorable dispersion characteristics, and lower thermal stability, suggesting potential utility in electronics, electrochemistry, biomedical applications, and the packaging and printing industries.

Mechanism

DHPM-generated shear forces and elevated pressure within a microenvironment selectively disrupt intermolecular hydrogen bonds in cellulose networks while preserving intramolecular hydrogen bonds, enabling uniform nanocellulose dispersion.

Bibliographic

Authors
Li J, Wang Y, Wei X, Wang F, Han D, Wang Q, et al.
Journal
Carbohydr Polym
Year
2014 (2014-11-26)
PMID
25256499
DOI
10.1016/j.carbpol.2014.06.085

Tags

Delivery context

The delivery route is not clearly identifiable from this paper. For hydrogen intake, inhalation is the most efficient route; inhalation, however, carries explosion risk (empirical LFL of 10%; high-concentration devices are not recommended).

Safety notes

The delivery route is not clearly identifiable from this paper. For hydrogen intake, inhalation is the most efficient route; inhalation, however, carries explosion risk (empirical LFL of 10%; high-concentration devices are not recommended).

See also:

Cite as: H2 Papers — PMID 25256499. https://h2-papers.org/en/papers/25256499
Source: PubMed PMID 25256499